Dataset: Measurements of the dissolved isotope radium-226 from samples collected on the US GEOTRACES GP17-OCE cruise on R/V Roger Revelle (RR2214) in the South Pacific and Southern Oceans from December 2022 to January 2023

ValidatedRelease Date:2026-09-13Final no updates expectedDOI: 10.26008/1912/bco-dmo.944841.1Version 1 (2024-12-11)Dataset Type:Cruise Results

Principal Investigator: Matthew A. Charette (Woods Hole Oceanographic Institution)

Co-Principal Investigator: Tristan J. Horner (Woods Hole Oceanographic Institution)

Scientist: Margot C.F. Debyser (Woods Hole Oceanographic Institution)

Technician: Paul B. Henderson (Woods Hole Oceanographic Institution)

BCO-DMO Data Manager: Shannon Rauch (Woods Hole Oceanographic Institution)


Program: U.S. GEOTRACES (U.S. GEOTRACES)

Project: US GEOTRACES GP17-OCE: Investigating the role of the Southern Ocean's biogeochemical divide in shaping the global distributions of radium and barium isotopes (GP17-OCE Ra and Ba isotopes)

Project: US GEOTRACES GP17-OCE and GP17-ANT: Sources and Rates of Trace Element and Isotope Cycling Derived from the Radium Quartet (GP17-OCE and GP17-ANT Radium Isotopes)

Project: US GEOTRACES GP17 Section: South Pacific and Southern Ocean (GP17-OCE) (GP17-OCE)


Abstract

This dataset includes measurements of the dissolved isotope radium-226 in the South Pacific and Southern Ocean. Samples were collected on the US GEOTRACES GP17-OCE cruise (Papeete, Tahiti to Punta Arenas, Chile) on R/V Roger Revelle from December 2022 to January 2023. Radium-223, radium-224, and radium-228 data will be made available in the future.

At sea, Radium-226 samples were collected following the GEOTRACES cookbook. Samples were collected from a 30-liter (L) Niskin mounted directly above a McLane large volume in situ pump WTS-LV (>1000 meters) or on the ODF CTD Rosette (<1000 meters). These samples (10-25 L) were recirculated through 20 grams (g) of manganese (Mn) oxide impregnated acrylic fiber at approximately <1 liter per minute (L/min) using small pumps. The Mn fibers from the Niskin bottles were rinsed with deionized water back at Woods Hole Oceanographic Institution (WHOI), partially dried, and sealed within a fiber holder after being flushed with helium equivalent to 30 column volumes. Samples were stored for a minimum of 12 days and analyzed for 226Ra via 222Rn ingrowth using alpha scintillation counting (Key et al., 1979). Samples were counted for 1-20 hours depending on the activity on the fiber, which resulted in counting uncertainties of ~2% dependent upon 226Ra content on the fiber and sample volume.


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Methods

Key, R. M., Brewer, R. L., Stockwell, J. H., Guinasso, N. L., & Schink, D. R. (1979). Some improved techniques for measuring radon and radium in marine sediments and in seawater. Marine Chemistry, 7(3), 251–264. doi:10.1016/0304-4203(79)90042-2